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Near-field Localization in Plasmonic Superfocusing: a Nanoemitter on a Tip

Journal Article · · Nano Letters, 10(2):592–596
DOI:https://doi.org/10.1021/nl903574a· OSTI ID:972523

The effective focusing of light to sub-wavelength dimensions has been a long standing desire in optics, yet proven challenging even resorting to a multitude of new strategies based on near-field effects, surface plasmon polaritons, and metamaterials1-7. The propagation of surface plasmon polaritons (SPP) on a conical tip to obtain nanoconfined light as proposed theoretically has recently emerged as a particularly promising candidate5-10. On the basis of our previous work, having established coupling of SPPs onto gold metal tips and their radiationless transport11, here, using a refined geometry we provide direct evidence of plasmonic nanofocusing into a localized excitation at the apex. As demonstrated by employing scattering-type scanning near-field optical microscopy (s-SNOM) efficient convergence of the optical fields into the 20 nm size apex volume is shown, exceeding the diffraction limit by more than one order of magnitude. The resulting nanoemitter is a point-like axial dipole with corresponding spectral and angular radiative characteristics. The associated linear and nonlinear field concentration as enabled by the unique 3D topology of the conical tip opens up exciting new applications in nano-optics, facilitating ultra-high spatio-temporal optical imaging, attosecond XUV generation, or antenna-based sensing and energy harvesting.

Research Organization:
Pacific Northwest National Laboratory (PNNL), Richland, WA (US), Environmental Molecular Sciences Laboratory (EMSL)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC05-76RL01830
OSTI ID:
972523
Report Number(s):
PNNL-SA-65996; 26701; KP1704020
Journal Information:
Nano Letters, 10(2):592–596, Journal Name: Nano Letters, 10(2):592–596 Journal Issue: 2 Vol. 10
Country of Publication:
United States
Language:
English

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