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Quantum and quasiclassical reactive scattering of O({sup 1}D)+HCl using an ab initio potential.

Journal Article · · Chem. Phys. Lett.
We report quasiclassical trajectory and quantum wavepacket calculations for the reaction of O({sup 1}D)+HCl using a recent ab initio potential energy surface. The quantum calculations, done only for zero total angular momentum and HCl(v=j=0), agree well with corresponding trajectory results in terms of total reactivity and the ClO/OH branching ratio. Quasiclassical trajectory cross-sections to final vibrational states of the OH and ClO products, the ClO/OH branch.
Research Organization:
Argonne National Laboratory (ANL)
Sponsoring Organization:
SC
DOE Contract Number:
AC02-06CH11357
OSTI ID:
942719
Report Number(s):
ANL/CHM/JA-33964
Journal Information:
Chem. Phys. Lett., Journal Name: Chem. Phys. Lett. Journal Issue: 3-4 ; Dec. 24, 1999 Vol. 315; ISSN CHPLBC; ISSN 0009-2614
Country of Publication:
United States
Language:
ENGLISH

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