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Magnetic switching and phase competition in the multiferroic antiferromagnet Mn1−xFexWO4

Journal Article · · Physical Review B
 [1];  [2];  [1];  [1];  [3];  [4];  [4];  [1];  [4]
  1. ORNL
  2. Argonne National Laboratory (ANL)
  3. National Institute of Standards and Technology (NIST)
  4. University of Houston, Houston
Elastic neutron scattering is used to study the spin correlations in the multiferroic Mn1−xFexWO4 with x=0.035, 0.05, and 0.10. The noncollinear incommensurate ICM magnetic structure associated with the ferroelectric FE phase in pure MnWO4 is suppressed at x=0.035 and completely absent at x=0.10. The ICM spin order and FE phase can be restored by applying a magnetic field along the spin easy axis. The low-T commensurate magnetic structure extends in both H/T with increasing Fe concentration. The systematic evolution of the magnetic and electric properties indicates that the noncollinear ICM spin order results from competing magnetic interactions and its stabilization can be tuned by the internal x or external magnetic-field perturbations.
Research Organization:
Oak Ridge National Laboratory (ORNL); High Flux Isotope Reactor
Sponsoring Organization:
SC USDOE - Office of Science (SC)
DOE Contract Number:
AC05-00OR22725
OSTI ID:
941608
Journal Information:
Physical Review B, Journal Name: Physical Review B Journal Issue: 19 Vol. 78
Country of Publication:
United States
Language:
English

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