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Microstructure Evolution and Grain Growth Kinetics in Annealed Nanocrystalline Chromium

Journal Article · · Journal of Physical Chemistry
DOI:https://doi.org/10.1021/jp066993q· OSTI ID:931912
 [1];  [1];  [1];  [2];  [2];  [2];  [3];  [4]
  1. Warsaw University
  2. University of Saarbrucken, Saarbrucken, Germany
  3. European Synchrotron Radiation Facility (ESRF)
  4. ORNL

The kinetics of thermal evolution of the microstructure of nanocrystalline chromium (nano-Cr) has been studied by time-resolved synchrotron radiation techniques: high-resolution powder diffraction and small-angle X-ray scattering (SAXS). The as-prepared electrodeposited nano-Cr with average grain size of 27 nm shows the same bcc structure as {alpha}-Cr. The nano-Cr cubic lattice parameter thermal expansion is the same as that of reference polycrystalline {alpha}-Cr. Annealing of nano-Cr at temperatures above 400 C leads to a grain growth process with the final grain size not exceeding 125 nm even at a temperature of 700 C. The single power-law behavior is observed by SAXS in as-prepared nano-Cr changes during annealing above 400 C. In nano-Cr samples annealed at temperatures between 400 and 700 C, the low-q part of the SAXS signal shows a Porod-type behavior while the high-q part shows a power-law Q-{alpha} with the exponent {alpha} < 4. This effect is probably due to changes of the grain surface roughness during grain growth.

Research Organization:
Oak Ridge National Laboratory (ORNL)
Sponsoring Organization:
SC USDOE - Office of Science (SC)
DOE Contract Number:
AC05-00OR22725
OSTI ID:
931912
Journal Information:
Journal of Physical Chemistry, Journal Name: Journal of Physical Chemistry Journal Issue: 111 Vol. 10.1021; ISSN JPCHAX; ISSN 0022-3654
Country of Publication:
United States
Language:
English

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