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Seeded Growth of Highly Luminescent CdSe/CdS Nano-Heterostructures with Rod and Tetrapod Morphologies

Journal Article · · Nano Letters
OSTI ID:928955

We have demonstrated that seeded growth of nanocrystals offers a convenient way to design nanoheterostructures with complex shapes and morphologies by changing the crystalline structure of the seed. By using Use nanocrystals with wurtzite and zinc blende structure as seeds for growth of US nanorods, we synthesized CdSe/CdS heterostructure nanorods and nanotetrapods, respectively. Both of these structures showed excellent luminescentproperties, combining high photoluminescence efficiency (similar to 80 and similar to 50percent for nanorods and nanotetrapods, correspondingly), giant extinction coefficients (similar to 2 x 10(7) and similar to 1.5 x 10(8) M-1 cm (-1) at 350 nm for nanorods and nanotetrapods, correspondingly), and efficient energy transfer from the US arms into the emitting CdSe Core.

Research Organization:
Ernest Orlando Lawrence Berkeley National Laboratory, Berkeley, CA (US)
Sponsoring Organization:
Materials Sciences Division
DOE Contract Number:
AC02-05CH11231
OSTI ID:
928955
Report Number(s):
LBNL-277E
Journal Information:
Nano Letters, Journal Name: Nano Letters Journal Issue: 10 Vol. 7
Country of Publication:
United States
Language:
English

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