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Fabrication and Performance of Ni-YSZ Anode Supported Cell for Coal Derived Syngas Application by Tape Casting and Spin Coating

Conference ·
OSTI ID:927404

Ni-YSZ anode supported cell has been developed for direct utilization of coal derived syngas as fuel in the temperature range of 700-850° C. The porous Ni-YSZ anode substrate was prepared based on processes of slip casting and lamination of anode tape. Then thin-film YSZ electrolyte was deposited on pre-sintered anode substrate via a colloidal spin coating technique and an optimized final sintering route. Dense and crackfree YSZ electrolyte was successfully obtained after sintering at 1440C for 4hrs. Processing factors like pre-sintering of anode, solvent, coating cycles and sintering route on the final properties of YSZ film was studied. A power density of 0.62W/cm2 has been achieved for the anode supported cell tested in 97%H2/3%H2O at 800°C. EIS test results indicated the cell performance was essentially influenced by interfacial resistance and charge transfer process.

Research Organization:
West Virginia University, Morgantown, WV; National Energy Technology Laboratory (NETL), Pittsburgh, PA, and Morgantown, WV
Sponsoring Organization:
U.S. DOE - Experimental Program to Stimulate Competitive Research (DOE EPSCoR); West Virginia University, Morgantown, WV
DOE Contract Number:
FG02-06ER46299
OSTI ID:
927404
Report Number(s):
DOE/NETL-IR-2008-011
Country of Publication:
United States
Language:
English