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Motif based Hessian matrixfor ab initio geometry optimization ofnanostructures

Journal Article · · Physical Review B
A simple method to estimate the atomic degree Hessian matrixof a nanosystem is presented. The estimated Hessian matrix, based on themotif decomposition of the nanosystem, can be used to accelerate abinitio atomic relaxations with speedups of 2 to 4 depending on the sizeof the system. In addition, the programing implementation for using thismethod in a standard ab initio package is trivial.
Research Organization:
Ernest Orlando Lawrence Berkeley NationalLaboratory, Berkeley, CA (US)
Sponsoring Organization:
USDOE Director. Office of Science. Advanced ScientificComputing Research
DOE Contract Number:
AC02-05CH11231
OSTI ID:
926286
Report Number(s):
LBNL--59974; BnR: KJ0101030
Journal Information:
Physical Review B, Journal Name: Physical Review B Journal Issue: 19 Vol. 73
Country of Publication:
United States
Language:
English

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