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Novel Regenerable Sodium Based Sorbents for CO2 Capture at Warm Gas Temperatures

Journal Article · · Energy and Fuels
DOI:https://doi.org/10.1021/ef070008v· OSTI ID:916957
A novel sorbent consisting of NaOH/CaO was developed for CO2 capture at 315 °C suitable for high-temperature CO2-capture applications, such as coal gasification systems. The sorbent is regenerable at 700 °C, and steam does not affect the sorbent performance. A multicycle test conducted in the atmospheric reactor at 315 °C indicated that the sorbent improved the performance with an increased number of cycles. The sorbent can also capture CO2 at a wide range of temperatures from ambient to 500 °C. However, the mechanism of CO2 capture is different at ambient temperature. The sorbent is unique because it has a high CO2-capture capacity of more than 3 mol/kg at 315 °C and is regenerable at 700 °C
Research Organization:
National Energy Technology Laboratory (NETL), Pittsburgh, PA, Morgantown, WV, and Albany, OR (United States)
Sponsoring Organization:
USDOE - Office of Fossil Energy (FE)
OSTI ID:
916957
Report Number(s):
DOE/NETL-IR-2007-212
Journal Information:
Energy and Fuels, Journal Name: Energy and Fuels Journal Issue: 4 Vol. 21; ISSN 0887-0624
Publisher:
American Chemical Society
Country of Publication:
United States
Language:
English

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