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Orientated Crystallization in Discontinuous Aramid Fiber/isotactic Polypropylene Composites under Shear Flow Conditions

Journal Article · · J. Appl. Polym. Sci.
DOI:https://doi.org/10.1002/app.21926· OSTI ID:913901
Melt blends of short aramid fibers (AF) and isotactic polypropylene (iPP) are subjected to shear at 145 C and the structural evolution and final morphology are examined by in situ synchrotron X-ray scattering/diffraction and high-resolution scanning electron microscopy, respectively. The results indicate that the presence of short AFs significantly enhances the crystallization of iPP. It is argued that shear flow in this system exerts a twofold orientating action, namely, on the bulk iPP molecules and on the short AFs. The resultant crystalline morphology reflects the combined effects of crystallization on orientated iPP molecules to facilitate a shish kebab morphology and at the interface of the aligned fibers, to form transcrystallinity.
Research Organization:
Brookhaven National Laboratory (BNL) National Synchrotron Light Source
Sponsoring Organization:
Doe - Office Of Science
DOE Contract Number:
AC02-98CH10886
OSTI ID:
913901
Report Number(s):
BNL--78469-2007-JA
Journal Information:
J. Appl. Polym. Sci., Journal Name: J. Appl. Polym. Sci. Vol. 98; ISSN 0021-8995; ISSN JAPNAB
Country of Publication:
United States
Language:
English