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Increasing PCB Radiolysis Rates in Transformer Oil

Journal Article · · Radiation Physics & Chemistry
The kinetics of Aroclor 1242 radiolysis in transformer oil, using high-energy electrons, was found to be analogous to that previously measured for individual polychlorinated biphenyl (PCB) congeners irradiated with ó-rays. The plot of the pseudo-first-order rate constant for PCB decomposition versus initial PCB concentration is a power function, with high rate constants for low concentrations. The addition of alkaline isopropanol to transformer oil was found to increase the pseudo-first-order rate constant for PCB decomposition. The rate constant under these conditions is independent of concentration. This may be explained by the establishment of chain reaction dechlorination in the oil.
Research Organization:
Idaho National Laboratory (INL)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC07-99ID13727
OSTI ID:
912054
Report Number(s):
INEEL/JOU-01-00469
Journal Information:
Radiation Physics & Chemistry, Journal Name: Radiation Physics & Chemistry Journal Issue: 4-5 Vol. 65
Country of Publication:
United States
Language:
English

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