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Stimulated Terahertz Emission from Intra-Excitonic Transitions inCu2O

Journal Article · · Physical Review Letters
OSTI ID:908462
We report the first observation of stimulated emission of terahertz radiation from internal transitions of excitons. The far-infrared electromagnetic response of Cu{sub 2}O is monitored via broadband terahertz pulses after ultrafast resonant excitation of three-dimensional 3p excitons. Stimulated emission from the 3p to the energetically lower 2s bound level occurs at a photon energy of 6.6 meV, with a cross section of {approx} 10{sup 14} cm{sup 2}. Simultaneous excitation of both exciton levels, in turn, drives quantum beats which lead to efficient terahertz emission sharply peaked at the difference frequency.
Research Organization:
Ernest Orlando Lawrence Berkeley NationalLaboratory, Berkeley, CA (US)
Sponsoring Organization:
USDOE Director. Office of Science. Office of Basic EnergySciences; Alexander von Humboldt Foundation
DOE Contract Number:
AC02-05CH11231
OSTI ID:
908462
Report Number(s):
LBNL--58459; BnR: KC0202020
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Vol. 96; ISSN 0031-9007; ISSN PRLTAO
Country of Publication:
United States
Language:
English

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