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Comment on the accuracy of Wertheim`s theory of associating fluids

Journal Article · · Journal of Chemical Physics
DOI:https://doi.org/10.1063/1.470036· OSTI ID:90482
;  [1]; ;  [2]
  1. School of Chemical Engineering, Cornell University, Ithaca, New York 14853 (United States)
  2. Department of Chemical Engineering, University of Wisconsin, Madison, Wisconsin 53706 (United States)

The results of recently developed Monte Carlo methods for simulation of strongly associating fluids show an apparent disagreement with Wertheim`s theory of associating fluids. In this comment we show that the disagreement observed arises largely from approximations used for the reference-fluid pair distribution function required by the theory. {copyright} {ital 1995} {ital American} {ital Institute} {ital of} {ital Physics}.

DOE Contract Number:
FG02-88ER13974
OSTI ID:
90482
Journal Information:
Journal of Chemical Physics, Journal Name: Journal of Chemical Physics Journal Issue: 9 Vol. 103; ISSN JCPSA6; ISSN 0021-9606
Country of Publication:
United States
Language:
English