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Optimization of mode-I fracture toughness of high-performance epoxies by using designed core-shell rubber particles

Conference ·
OSTI ID:76237
;  [1]; ;  [2]
  1. Texas Polymer Center, Freeport, TX (United States)
  2. Dow Chemical Co., Midland, MI (United States)

The fracture behavior of high-performance epoxies modified with seven types of designed core-shell rubber particles is examined by using various microscopic techniques. The mode-I plane-strain fracture-toughness values (K{sub Ic}) of the designed rubber-modified epoxy systems that have highly cross-linked epoxy vary with the architecture of the interface between the matrix and the rubber particles. Accordingly, the toughening mechanisms observed among these systems are very different: rubber-particle cavitation and matrix shear yielding are found in systems that exhibit higher K{sub Ic} values; only crack deflection is found in systems that possess lower K{sub Ic} values. Synergistic toughening can be obtained if both the matrix shear-yielding and the crack-deflection mechanisms are operative upon fracture. An approach for toughening highly cross-linked epoxies is addressed. 67 refs., 18 figs., 2 tabs.

OSTI ID:
76237
Report Number(s):
CONF-900802--
Country of Publication:
United States
Language:
English

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