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Title: Radionuclide characterization of reactor decommissioning waste and neutron-activated metals

Technical Report ·
OSTI ID:7368473

This study is providing the NRC and licensees with a more comprehensive data base for regulatory assessment of the radiological factors associated with reactor decommissioning and disposal of wastes generated during these activities. The objectives of this study are being accomplished during the actual decommissioning of Shippingport Station and the detailed analysis of neutron-activated materials from commercial reactors. The radiological characterization studies of Shippingport decommissioning materials have now been completed, and analyses of dismantled piping and scabbled concrete have shown that neutron activation products, dominated by Co-60, comprised the residual radionuclide inventory. Waste classification assessment have shown that all decommissioning materials (except reactor pressure vessel internals) could be disposed of as Class A waste. Spent fuel disassembly hardware from the Shippingport Core-3 was analyzed for long-lived activation products. Nb-94 and Ni-63 concentrations in Inconel-X750 and stainless steel components exceeded their Class C limits. Measurements and assessments of C-14 in spent fuel disassembly hardware from three commercial nuclear power stations showed that this radionuclide never exceeded the Class C limit for al components. However, the Ni-63 and Nb-94 concentrations in some of these materials did exceed the Class C limits. These measurements are providing the basis for an assessment of the disposal options for these types of highly radioactive materials. Work is continuing on radiological characterization of spent PWR and BWR control rod assemblies. Three control rods, including a BWR cruciform control rod blade, a PWR control rod cluster assembly, and a PWR burnable poison rod assembly, have been characterized for their long-lived activation product concentrations and distribution by direct assay methods. These spent control rods could all be classified as Class C low-level waste. These rods are presently being sampled.

Research Organization:
Pacific Northwest Lab., Richland, WA (United States)
Sponsoring Organization:
USNRC; Nuclear Regulatory Commission, Washington, DC (United States)
DOE Contract Number:
AC06-76RL01830
OSTI ID:
7368473
Report Number(s):
NUREG/CR-5894; PNL-8106; ON: TI93016280
Country of Publication:
United States
Language:
English

Related Subjects

22 GENERAL STUDIES OF NUCLEAR REACTORS
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES
BWR TYPE REACTORS
DECOMMISSIONING
LWBR TYPE REACTORS
PWR TYPE REACTORS
RADIOACTIVE WASTE DISPOSAL
PLANNING
SHIPPINGPORT REACTOR
CALVERT CLIFFS-1 REACTOR
CARBON 14
COBALT 60
CONCRETES
CONTAMINATION REGULATIONS
CONTROL ELEMENTS
COOPER REACTOR
EXPERIMENTAL DATA
GAMMA SPECTROSCOPY
INCONEL ALLOYS
IRON 53
LOW-LEVEL RADIOACTIVE WASTES
NICKEL 63
NIOBIUM 94
PIPES
POINT BEACH-1 REACTOR
QUALITATIVE CHEMICAL ANALYSIS
RADIOACTIVE WASTES
RADIOASSAY
SAMPLING
SILVER 108
SILVER 110
SPENT FUELS
STAINLESS STEELS
US NRC
ALLOYS
BETA DECAY RADIOISOTOPES
BETA-MINUS DECAY RADIOISOTOPES
BETA-PLUS DECAY RADIOISOTOPES
BREEDER REACTORS
BUILDING MATERIALS
CARBON ISOTOPES
CHEMICAL ANALYSIS
COBALT ISOTOPES
DATA
DAYS LIVING RADIOISOTOPES
ELECTRON CAPTURE RADIOISOTOPES
ENERGY SOURCES
ENRICHED URANIUM REACTORS
EVEN-EVEN NUCLEI
EVEN-ODD NUCLEI
FUELS
HIGH ALLOY STEELS
INFORMATION
INTERMEDIATE MASS NUCLEI
INTERNAL CONVERSION RADIOISOTOPES
IRON ALLOYS
IRON BASE ALLOYS
IRON ISOTOPES
ISOMERIC TRANSITION ISOTOPES
ISOTOPES
LIGHT NUCLEI
MANAGEMENT
MATERIALS
MINUTES LIVING RADIOISOTOPES
NATIONAL ORGANIZATIONS
NICKEL ALLOYS
NICKEL BASE ALLOYS
NICKEL ISOTOPES
NIOBIUM ISOTOPES
NUCLEAR FUELS
NUCLEI
NUMERICAL DATA
ODD-ODD NUCLEI
POLLUTION REGULATIONS
POWER REACTORS
RADIOACTIVE MATERIALS
RADIOACTIVE WASTE MANAGEMENT
RADIOISOTOPES
REACTOR COMPONENTS
REACTOR MATERIALS
REACTORS
REGULATIONS
SECONDS LIVING RADIOISOTOPES
SILVER ISOT
SILVER ISOTOPES
SPECTROSCOPY
STEELS
THERMAL REACTORS
US ORGANIZATIONS
WASTE DISPOSAL
WASTE MANAGEMENT
WASTES
WATER COOLED REACTORS
WATER MODERATED REACTORS
YEARS LIVING RADIOISO
YEARS LIVING RADIOISOT
YEARS LIVING RADIOISOTOPES
220900* - Nuclear Reactor Technology- Reactor Safety
210100 - Power Reactors
Nonbreeding
Light-Water Moderated
Boiling Water Cooled
210200 - Power Reactors
Nonbreeding
Light-Water Moderated
Nonboiling Water Cooled
210500 - Power Reactors
Breeding
052002 - Nuclear Fuels- Waste Disposal & Storage