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Biological pathways and chemical behavior of plutonium and other actinides in the environment

Journal Article · · ACS Symp. Ser.; (United States)
The principal long-lived actinide elements that may enter the environment from either U or Pu fuel cycles are Pu, Am, Cm, and Np. Approximately 25% of the alpha activity estimated to be released to the atmosphere from the LMFBR fuel cycle will be contributed by /sup 241/Am, /sup 242/Cm, and /sup 244/Cm. The balance of the alpha activity will come from Pu isotopes. Activities of /sup 242/Cm, /sup 244/Cm, /sup 241/Am, /sup 243/Am, and /sup 237/Np in waste may exceed concentrations of Pu isotopes in waste after various periods of decay. Thorium and uranium isotopes may also be released by operations of the thorium fuel cycle. Environmental actinides are discussed under the following headings: sources of man-made actinide elements; pathways of exposure; environmental chemistry of actinides; uptake of actinides by plants; distribution of actinides in components of White Oak Lake; entry of actinides into terrestrial food chains; relationship between chemical behavior and uptake of actinides by organisms; and behavior of Pu in freshwater and marine food chains. (HLW)
Research Organization:
Oak Ridge National Lab., TN
OSTI ID:
7292490
Journal Information:
ACS Symp. Ser.; (United States), Journal Name: ACS Symp. Ser.; (United States) Vol. 35; ISSN ACSMC
Country of Publication:
United States
Language:
English