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Thermodynamics of oxygen and nitrogen in liquid nickel equilibrated with CaO-TiO[sub x] and CaO-TiO[sub x]-Al[sub 2]O[sub 3] melts

Journal Article · · Metallurgical Transactions, B (Process Metallurgy); (United States)
OSTI ID:7284061
Equilibrium between CaO-TiO[sub x] or CaO-TiO[sub x]-Al[sub 2]O[sub 3] slags and liquid nickel with respect to oxygen and nitrogen has been studied at 1873 K as a function of Ti (or Al) content in metal, using lime and alumina crucibles. The Al-O, Ti-O, and Ti-Al relations were obtained for liquid nickel equilibrated with these slags. Nitride capacity, C[sub (N)], defined by (mass pct N)[center dot] P[sub O[sub 2]][sup 3/4]/P[sub N[sub 2]][sup 1/2], was evaluated from nitrogen distribution ratios, L[sub N] [l brace]= (mass pct N)/[mass pct N][r brace], coupled with oxygen content in liquid nickel. Activities of Al[sub 2]O[sub 3] and activity coefficients of TiO[sub 2] and TiO[sub 1.5] were estimated either from the content of Al, Ti, and O, using the compiled data for the free energy of formation of oxide and the respective interaction parameters or from the values for L[sub N] and C[sub (N)].
OSTI ID:
7284061
Journal Information:
Metallurgical Transactions, B (Process Metallurgy); (United States), Journal Name: Metallurgical Transactions, B (Process Metallurgy); (United States) Vol. 25:1; ISSN MTTBCR; ISSN 0360-2141
Country of Publication:
United States
Language:
English

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