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Structural effect in neutron irradiation of insulating ceramics

Conference ·
OSTI ID:7269287

A vacuum gap irradiation capsule was designed and built to maintain a temperature of 740/sup 0/C during 6 weeks irradiation at EBR-II. Sixty-eight samples of 15 ceramic or metal-ceramic combinations were irradiated to a fluence of approximately 3 x 10/sup 21/ neutrons/cm/sup 2/, E greater than 0.1 MeV. Measurements of sample dimensions before and after irradiation were used to determine volume swelling. This parameter and the physical appearance of the samples are discussed. A primary application of insulating ceramics in proposed fusion powder devices is the first wall insulating lining in the RTPR reactor. A satisfactory material for this application must bear substantial thermal stresses in cyclical fashion. Calculated values of pertinent parameters are presented and compared for several of the irradiated materials in non-irradiated form. Work to prepare apparatus for the measurement of thermal and mechanical properties of these materials following neutron irradiation is described. Silicon nitride is representative of a class of refractory ceramics distinguished by its high thermal conductivity, resistance to thermal shock, and elevated temperature strength retention. Recent work has suggested that Si/sub 3/N/sub 4/ hot pressed with additions of Y/sub 2/O/sub 3/, rather than the usual MgO, may offer improved high temperature strength. A project to prepare samples of this material with optimized Y/sub 2/O/sub 3/ concentration and pressing conditions is described. Samples of Si/sub 3/N/sub 4/ hot pressed with 0, 5, 10, 15, and 20 wt percent Y/sub 2/O/sub 3/ additions have been prepared for an irradiation experiment being carried out by ORNL at EBR-II.

Research Organization:
Los Alamos Scientific Lab., N.Mex. (USA)
DOE Contract Number:
W-7405-ENG-36
OSTI ID:
7269287
Report Number(s):
LA-UR-76-1131; CONF-760558-1
Country of Publication:
United States
Language:
English

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