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Title: The epitaxial growth and magnetic analysis of ultrathin films of iron/silver and iron/nickel

Miscellaneous ·
OSTI ID:7236545

The first part of these thesis concerns Fe(110)/Ag(111) multilayers, the second investigates the Fe(100)/Ag(100) system and the last examines Fe/bcc Ni multilayers. All films were grown using molecular beam epitaxy, examined for in-plane crystalline structure using in situ reflection high energy electron diffraction, and their magnetic properties were deduced using Moessbauer spectroscopy. The Fe/bcc Ni films were also investigated with x-ray diffraction and fluorescence, and three types of magnetometries. Fe(110)/Ag(111) multilayers were grown, with the Fe layer 3 monolayers thick and the Ag thickness from 4 to 20 ML. For thin Ag spacers, the Fe layers communicated magnetically and gave rise to a T[sup 3/2] dependence. As the Fe layers were separated by thicker Ag layers, they acted more as 2-D ferromagnets and showed a more linear dependence. Another series of films was grown to analyze the B-value of surface spin waves when this Fe surface was separated from another Fe layer. The B-value of the spinwaves exhibited apparent oscillations at separation distances of 5-6 ML. The typical doubling in B-value was seen at the surface. A series of Fe(100)/Ag(100) multilayers were grown on rock salt substrates. Demonstrating a large quadrupole splitting and three different Fe sites, it was postulated that the three sites corresponded to a bulk-like site, a Fe/Ag interface, and a Ag/Fe interface. An [sup 57]Fe probe layer was placed in each of these sites in three different films. The different sites were approximately resolved. Two series of Fe(110)/bcc Ni(110) and Fe(100)/bcc Ni(100) multilayers were grown. RHEED inferred that the Ni grew in a metastable phase of bcc Ni in both orientations. SQUID showed that the (110) type had an order-of-magnitude lower coercivity than the (100). Magnetometry implied that bcc Ni overlayers on Fe with thicknesses of 8 ML and greater are ferromagnetic at room temperature.

Research Organization:
Johns Hopkins Univ., Baltimore, MD (United States)
OSTI ID:
7236545
Resource Relation:
Other Information: Thesis (Ph.D.)
Country of Publication:
United States
Language:
English