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A critical review of measurements of the unattached'' fraction of the radon decay products

Technical Report ·
OSTI ID:7189645

Exposure to radon and its decay products is known to cause lung cancer. It is the deposition of the decay products within the respiratory tract that delivers the dose leading to adverse health effects. An important concept in understanding the health effects of the radon progeny is the unattached'' fraction. It was suggested that there is a highly diffusive form of the radon and thoron decay products that can be fully deposited in the respiratory system referred to as the unattached fraction.'' Initial measurements were made using diffusional deposition in tubes to separate the high diffusivity unattached'' activity from that associated with lower diffusion coefficient particles. Subsequently, wire screens were used to estimate unattached'' Rn daughter fractions in ambient and mine atmospheres. Wire screen penetration theory along with a semi-empirically corrected diffusion coefficient equation can be used to characterize the previously reported unattached'' fraction measurements. Collection efficiency curves have been estimated for previously published wire screen unattached'' fraction measurements and the measurements available in the literature are reviewed and discussed. The purpose for measuring unattached fraction is to estimate the dose to the respiratory tract arising from the deposition of radon decay products to which the individual is exposed. Therefore, if measurements could be made in a manner that better reflected the aerodynamic behavior of the radon progeny in the respiratory tract, then the assessment of exposure could be directly related to dose with far greater accuracy. Respiratory deposition models can serve as basis for such a system and the design concepts of such a measurement system is presented. 104 refs., 34 figs., 7 tabs.

Research Organization:
Clarkson Coll. of Tech., Potsdam, NY (USA). Dept. of Chemistry
Sponsoring Organization:
DOE/ER
DOE Contract Number:
FG02-89ER60876
OSTI ID:
7189645
Report Number(s):
DOE/ER-0451P; ON: DE90010157
Country of Publication:
United States
Language:
English