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Evaluation of springtime nitrogen oxide and oxidant data from a suburban/rural northeast USA surface site. [PRECP]

Conference ·
OSTI ID:7126615

Full characterization of the air chemistry (gases, particles and meteorology) was accomplished for a rural site in Bucks County, PA during April 1985, in connection with PRECP field experiments. Data from continuous monitoring of nitrogen oxides (NO/sub y/), nitric acid, ozone and SO/sub 2/ are used in this evaluation along with PAN analyses every 30 min, meteorological data from surface observations and a single theodolite radiosonde system, and selected aerosol compositions and gaseous aldehyde data. Limited precipitation composition data from a manual sequential sampler is available including common ions, dissolved SO/sub 2/ and H/sub 2/O/sub 2/. Correlation matrices, averaged diurnal trends, and pollution roses will be presented indicating strong relationships between ozone and the secondary nitrogen oxide species, HNO/sub 3/ and PAN. Periods of impact from the greater Philadelphia and New York source regions can be identified from NO/sub y/ and SO/sub 2/ data, but anticyclonic flow in aged air masses advected from the west resulted in the major importation of secondary nitrogen(V) and sulfur(VI) species (HNO/sub 3/, PAN and aerosol sulfate) to this site. 16 refs.

Research Organization:
Brookhaven National Lab., Upton, NY (USA); Los Alamos National Lab., NM (USA); Argonne National Lab., IL (USA)
DOE Contract Number:
AC02-76CH00016
OSTI ID:
7126615
Report Number(s):
BNL-41221; CONF-880912-3; ON: TI88009892
Country of Publication:
United States
Language:
English