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Radiation-enhanced corrosion of mild steel

Conference · · Trans. Am. Nucl. Soc.; (United States)
OSTI ID:7093501

A problem which may be encountered in high-level radioactive waste repositories in geological salt formations is the possibility of groundwater infiltrating the repository, dissolving the salt and forming a corrosive brine solution. This brine may then attack the steel overpack which surrounds the primary waste container. The presence of a high-level gamma radiation field has been known to significantly increase the rate of corrosion. The increased corrosion rate has been attributed to the formation of corrosive, oxidizing radiolysis products. The objective of this research was to study corroded metal surfaces to determine the type of corrosion (uniform, pitting, intergranular, etc.) that is taking place in a radiation field. An understanding of the corroded surface may yield some insight to the mechanisms that contribute to corrosion in a high-level waste repository. Immersion corrosion tests were conducted on Type 1018 mild steel. The steel coupons were immersed in deaerated solutions of sodium chloride and magnesium chloride. The solutions were of various compositions and concentrations ranging from 0% NaCl to 0% MgCl/sub 2/ to saturated solutions. Half of the immersion tests were conducted in a 60 Gy/min (6000 rad/min) /sup 60/Co gamma radiation field. The second half of the samples were placed in a low background area to act as a reference.

Research Organization:
Univ. of Virginia, Charlottesville
OSTI ID:
7093501
Report Number(s):
CONF-861102-
Journal Information:
Trans. Am. Nucl. Soc.; (United States), Journal Name: Trans. Am. Nucl. Soc.; (United States) Vol. 53; ISSN TANSA
Country of Publication:
United States
Language:
English