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Neutron scattering study of spin fluctuations in Y(Mn/sub 1-//sub x/Al/sub x/)/sub 2/

Journal Article · · Phys. Rev. B: Condens. Matter; (United States)

Elastic and inelastic neutron-scattering measurements have been made on a series of pseudobinary intermetallic compounds Y(Mn/sub 1-//sub x/Al/sub x/)/sub 2/. Long-range antiferromagnetic order below T/sub N/approx.100 K in YMn/sub 2/ has been shown to collapse by substitution of only 5% of the manganese atoms by aluminum atoms. In these compounds, a spin-glass transition has been clearly indicated by a change in the energy width of the scattered-neutron spectrum, as well as by the onset of field hysteresis in susceptibility measurements. In the compound with x = 0.10, the amplitude of spin fluctuations S does not change appreciably with temperature, whereas in YMn/sub 2/ it drops by more than 30% at T/sub N/ and then increases gradually with increasing temperature. A considerable degree of spatial correlations of spin fluctuations persists up to at least 760 K, which is similar to the behavior observed in YMn/sub 2/ but quite different from the characteristics of simple localized-electron magnets.

Research Organization:
Department of Physics, Faculty of Science, Saitama University, 255 Shimo-Okubo, Urawa, Saitama 338, Japan
OSTI ID:
7091976
Journal Information:
Phys. Rev. B: Condens. Matter; (United States), Journal Name: Phys. Rev. B: Condens. Matter; (United States) Vol. 38:7; ISSN PRBMD
Country of Publication:
United States
Language:
English