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Stability of alternate fuels

Journal Article · · Hydrocarbon Process.; (United States)
OSTI ID:7089393

Samples of gasoline and jet fuel produced from coal, oil shale, or tar sands were stored in amber glass bottles for 32 weeks at 43.3/sup 0/C (110/sup 0/F), and the amounts of gum formed in each were determined. Samples of petroleum-derived gasoline and jet fuel were stored under the same conditions for comparison with the alternate fuels. The petroleum-derived fuels showed good storage stability, while most of the synthetic fuels developed high levels of deposits after 32 weeks. Accelerated storage at 93.3/sup 0/C (200/sup 0/F) for 16 hours produced results that correlated well with the 43.3/sup 0/C, 32 week storage for the gasoline samples, but not for the jet fuels. HPLC and GC analyses of the samples before and after storage indicated that the gasolines lost some of the lighter components during storage, but the jet fuels showed very little change in composition with storage. IR and GPC analyses of the gums revealed a high concentration of oxygenated material and some high molecular weight material, indicating the gum formation is primarily the result of oxidation reactions with some polymerization. Elemental analyses showed that nitrogen and sulfur compounds tended to concentrate in the gum.

OSTI ID:
7089393
Journal Information:
Hydrocarbon Process.; (United States), Journal Name: Hydrocarbon Process.; (United States) Vol. 59:7; ISSN HYPRA
Country of Publication:
United States
Language:
English