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Production of Ba/sup +/ in a two-photon radiative collision in crossed Na-Ba beams

Journal Article · · Phys. Rev. A; (United States)

We report the observation of a two-step radiative collisional ionization between Na((3p /sup 2/P/sub 3/2/) and Ba(6s/sup 2/ /sup 1/S/sub 0/) in which an optical p photon is absorbed simultaneously with the collision, Na((3p /sup 2/P/sub 3/2/)+Ba(6s/sup 2/ /sup 1/S/sub 0/)+h..omega -->..Ba((6p/sup 2/ /sup 1/S/sub 0/)+Na(3s /sup 2/S/sub 1/2/) and with subsequent photoionization of the excited barium, Ba((6p/sup 2/ /sup 1/S/sub 0/)+h..omega -->..Ba/sup +/+e. We observe peak ion intensity close to the difference frequency between Ba((6p/sup 2/ /sup 1/S/sub 0/) and Na((3p /sup 2/P/sub 3/2/) as well as a quadratic increase of ion intensity with laser power. These results confirm, complement, and extend the interpretation of an earlier observation.

Research Organization:
Department of Chemistry, University of Maryland, College Park, Maryland 20742
OSTI ID:
7050992
Journal Information:
Phys. Rev. A; (United States), Journal Name: Phys. Rev. A; (United States) Vol. 29:4; ISSN PLRAA
Country of Publication:
United States
Language:
English