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Title: Polarization effects in the differential cross section of the Ba( sup 1 P sub 1 - sup 3 P sub 2 ) inelastic transition induced by argon

Journal Article · · Physical Review A. General Physics; (United States)
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  1. Service des Photons, Atomes et Molecules, Centre d'Etudes de Saclay, 91191 Gif-sur-Yvette CEDEX (France)

The Ba(6{ital s}6{ital p} {sup 1}{ital P}{sub 1}{r arrow}{sup 3}{ital P}{sub 2}) inelastic transition induced by argon has been investigated in a crossed beam as a function of the collision energy between 0.14 and 0.40 eV. The differential cross sections have been obtained by the Doppler technique probing the Ba(6{ital s}6{ital p} {sup 3}{ital P}{sub 2}) with a single-mode cw laser. Oscillations are observed in the differential cross sections that are assigned to Stueckelberg interferences resulting from a crossing between the {sup 1}{Pi}{sub 1} and {sup 3}{Sigma}{sub 1} Ba-Ar potential-energy curves. A very large polarization effect is observed by comparing the differential cross sections corresponding to a {ital p}{sigma} or a {ital p}{pi} preparation of the Ba({sup 1}{ital P}{sub 1}) orbital with respect to the relative Ba-Ar velocity.

OSTI ID:
7043657
Journal Information:
Physical Review A. General Physics; (United States), Vol. 45:9; ISSN 1050-2947
Country of Publication:
United States
Language:
English