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NMR study of ion-molecule interaction. 4. /sup 1/H and /sup 35/Cl NMR of chloride ion-trihalomethane association

Journal Article · · J. Phys. Chem.; (United States)
DOI:https://doi.org/10.1021/j100319a057· OSTI ID:7005251
Associations due to hydrogen bonding between chloride ion and trichloromethane or tribromomethane in carbon tetrachloride, acetonitrile, acetone, and N,N-dimethylformamide were investigated by using the /sup 1/H NMR chemical shift and the /sup 35/Cl NMR line width measurements. These measurements were used to obtain the proton shifts of the associated trihalomethanes, the line widths of the associated Cl/sup -/ ions, and the concentration equilibrium constants for associations between trihalomethanes and a Cl/sup -/ ion. The proton shifts of the associated trihalomethanes have a constant value regardless of the character of the solvent, whereas the line widths of the associated Cl/sup -/ ion show solvent dependence. The magnitude of the line width appears to be related to the dielectric constant of the solvent.
Research Organization:
Kitami Institute of Technology, Hokkaido (Japan)
OSTI ID:
7005251
Journal Information:
J. Phys. Chem.; (United States), Journal Name: J. Phys. Chem.; (United States) Vol. 92:8; ISSN JPCHA
Country of Publication:
United States
Language:
English

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