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Characteristics and behavior of emulsion at nuclear fuel reprocessing

Journal Article · · Nucl. Technol.; (United States)
OSTI ID:6993669

The characteristics and behavior of the emulsion formed in mixer-settlers during nuclear fuel reprocessing were studied with the dissolver solution of spent fuel burned up to 28,000 MWd/MTU and a palladium colloidal solution, respectively. The emulsion was observed to be oil in water where nonsoluble residues of spent fuel were condensed as emulsifiers. Emulsion formed at interfaces in the settler showed electric conductivity due to continuity of the aqueous phase of the emulsion and viscosity due to the creamy state of the emulsion. The higher the palladium particle concentration was, the larger the amount of emulsion formed. This result agreed well with experience obtained in the Tokai Reprocessing Plant operation that both nonsoluble residues and emulsion formation increased remarkably on fuels in which burnup exceeded 20 000 MWd/MTU.

Research Organization:
Power Reactor and Nuclear Fuel Development Corporation Tokai Reprocessing Plant, Operation Testing Laboratory Tokai, Ibaraki, 319-11
OSTI ID:
6993669
Journal Information:
Nucl. Technol.; (United States), Journal Name: Nucl. Technol.; (United States) Vol. 57:2; ISSN NUTYB
Country of Publication:
United States
Language:
English