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Small-angle x-ray scattering studies of crazed glassy polymers

Journal Article · · J. Polym. Sci., Polym. Phys. Ed.; (United States)

A small-angle x-ray scattering (SAXS) study of the relaxed craze structure in polystyrene was performed using the Oak Ridge National Laboratory 10-m SAXS facility. Coupled with known results from transmission electron microscopy studies, the SAXS patterns can be interpreted as scattering from an open-cell foam with void spaces interspersed among the fibrils. Results have shown the scattering centers in crazed polystyrene can be modeled as cylinders the axes of symmetry of which are parallel to the tensile axes. Scattering centers are bimodal in their size distribution, with aspect ratios of 1.0 and 2.6. Crazes in lower-molecular-weight polystyrene, while variations in strain rate and test temperature during craze formation have no effect on the relaxed craze morphology. A comparison of SAXS patterns from polystyrene and polycarbonate indicates that the morphologies of their respective crazes are significantly different.

Research Organization:
Univ. of Tennessee, Knoxville
OSTI ID:
6973164
Journal Information:
J. Polym. Sci., Polym. Phys. Ed.; (United States), Journal Name: J. Polym. Sci., Polym. Phys. Ed.; (United States) Vol. 21; ISSN JPLPA
Country of Publication:
United States
Language:
English