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Analysis of the Argonne premium coal samples by thermogravimetric Fourier transform infrared spectroscopy

Journal Article · · Energy and Fuels; (USA)
DOI:https://doi.org/10.1021/ef00021a017· OSTI ID:6960144
; ; ;  [1]; ; ; ;  [2]
  1. Advanced Fuel Research, Inc., Hartford, CT (USA)
  2. Bomem, Inc., Quebec City, Quebec (Canada)

The authors have developed a TG-FTIR instrument that combines thermogravimetric analysis (TGA) with evolved product analysis by Fourier transform infrared (FT-IR) spectroscopy. FT-IR analysis of evolved products has advantages over mass spectroscopy in allowing analysis of very heavy products and over gas chromatography in speed. This paper describes the most recent improvements in the apparatus and presents its application in characterizing the Argonne premium coal samples. The TG-FTIR apparatus for pyrolysis, oxidation of pyrolysis products, and oxidation of the sample is described. To analyze coal, a sequence of drying, pyrolysis, and combustion is employed to obtain proximate analysis, volatile composition, volatile kinetics, and relative char reactivity. Pyrolysis results are presented for the eight Argonne coals, several demineralized coals, and two oxidized samples of Pittsburgh Seam coal.

DOE Contract Number:
AC21-86MC23075
OSTI ID:
6960144
Journal Information:
Energy and Fuels; (USA), Journal Name: Energy and Fuels; (USA) Vol. 4:3; ISSN ENFUE; ISSN 0887-0624
Country of Publication:
United States
Language:
English