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Comparative behavior of americium and plutonium in wastewater

Conference · · Sov. Radiochem. (Engl. Transl.); (United States)
OSTI ID:6937505
This paper studies the behavior of trace americium and plutoniumin wastewater fed into purification systems. Activities of the elements were determined on a semiconductive alpha-ray spectrometer. the distributio nonuniformity, or heterogeneity, of americium and plutonium per unit volume of wastewater was determined quantitatively before and after passage through filter papers. The two elements were found to be in a colloidal or pseudocolloidal state in the original wastewater sample at pH 6. On acidifying the wastewater from pH 4 to 1 M nitric acid the americium passed quantitatively into the water phase but the most plutonium remained in the colloidal or pseudocolloidal state. the plutonium also passed quantitatively into the water phase in wastewater at a 1 M nitric acid acidity but only after a prolonged (12-day) hold. A knowledge of the heterogeneity of plutonium and americium in wastewaters made it possible to quickly distinguish their state, i.e., colloidal, pseudocolloidal, or in true solution.
OSTI ID:
6937505
Report Number(s):
CONF-8306297-
Conference Information:
Journal Name: Sov. Radiochem. (Engl. Transl.); (United States) Journal Volume: 28:1
Country of Publication:
United States
Language:
English