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Collection, analysis, and deposition of airborne organic pollutants

Thesis/Dissertation ·
OSTI ID:6918251

A commercial high-volume air sampler with a mixed adsorbent cartridge was evaluated for the collection of semivolatile organics with vapor pressures of 10/sup -3/-10/sup 0/ torr. An apparatus was built wherein vapors of chlorobenzenes, and naphthalenes, and biphenyl were diluted (mixed) with 30-165 m/sup 3/ of filtered and scrubbed laboratory air and then pulled through a polyurethane foam (PUF)-Tenax adsorbent cartridge with a PS-1 hi-vol sampler. The vapor penetration through the main trap was monitored with a back-up adsorbent cartridge. The test compounds were soxhlet extracted from the adsorbents and analyzed by capillary gas chromatography. Collection efficiency based on mass balance averaged 90% +/- 13% for p- and o-dichlorobenzenes, and 92% +/- 14% for hexachlorobenzene; the most-and least-volatile compounds tested. Overall, collections averaged 97% +/- 13%. The rainfall input of organochlorine pesticides and polychlorinated biphenyls (PCB) to a pristine South Carolina salt marsh was monitored with both bulk and wet-only collectors from July 1981-February 1983. Toxaphene was present in the highest average concentration, 28 ng/L in 31/40 samples, and was up to 80 times higher in summer rains than any other organochlorine analyzed. Both ..cap alpha..-HCH and ..gamma..-HCH were found in nearly every sample while PCB, chlordane, and DDT residues were each found in less than half of the samples.

Research Organization:
South Carolina Univ., Columbia (USA)
OSTI ID:
6918251
Country of Publication:
United States
Language:
English