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Interference in the angular cross section for photodissociation of metastable H sub 2

Journal Article · · Physical Review Letters; (USA)
; ;  [1]
  1. FOM-Institute for Atomic and Molecular Physics, Kruislaan 407, 1098 SJ Amsterdam, The Netherlands (NL)

The anisotropy of the photodissociation cross section of metastable H{sub 2} for excitation around the resonance due to the {sup 3}{Delta}{sub g}{sup {minus}}(v=5,{ital N}+2) level is investigated. The {ital j} {sup 3}{Delta}{sub {ital g}}{sup {minus}}({ital v}=5,{ital N}=2) state is coupled to the continuum of the {ital i} {sup 3}{Pi}{sub {ital g}}{sup {minus}} state by the nuclear rotation. Since both states carry oscillator strength, the cross section shows interference effects. The interference is difficult to detect on the total cross section, but is clearly seen in the angular distribution of the photofragments.

OSTI ID:
6903183
Journal Information:
Physical Review Letters; (USA), Journal Name: Physical Review Letters; (USA) Vol. 64:13; ISSN PRLTA; ISSN 0031-9007
Country of Publication:
United States
Language:
English