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Laser spectroscopic measurements of isotope shift and hyperfine structure in sup 207 Bi and sup 208 Bi

Thesis/Dissertation ·
OSTI ID:6903077

Measurements of the hyperfine spectra of 38-yr {sup 207}Bi and 3.7 {times} 10{sup 5} - yr {sup 208}Bi in the 6p{sup 3} {sup 4}S{sub 3/2} - 6p{sup 2}7s {sup 4}P{sub 1/2} 306.7-nm resonance line were made using laser spectroscopic methods. The atomic excitation was produced with use of the frequency doubled output of a tunable ring dye laser. Laser absorption spectroscopy was used for the {sup 208}Bi measurement, while fluorescence spectroscopy, with photon counting detection, was used for {sup 208}Bi. The experiments of {sup 207}Bi were performed in both zero and high (0.7515 T) magnetic fields. The latter also provided a reliable measurement of the nuclear spin of {sup 207}Bi. The isotope shift odd-even staggering parameter for {sup 208}Bi, {gamma} = 0.752(43), was derived and used for an isotonic comparison. The measured nuclear magnetic moments are in agreement with theoretical predictions. An improved calculation of the isotope shift constant using a diffuse nuclear charge model is given and a weak, but significant, model dependence of the isotope shifts was found.

Research Organization:
New York Univ., NY (USA)
OSTI ID:
6903077
Country of Publication:
United States
Language:
English