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Spin-specific photoelectron diffraction using magnetic x-ray circular dichroism

Journal Article · · Journal of Applied Physics; (United States)
DOI:https://doi.org/10.1063/1.358225· OSTI ID:6836554
;  [1]; ;  [2]
  1. Department of Chemistry and Materials Science, Lawrence Livermore National Laboratory, Livermore, California 94550 (United States)
  2. Laboratory for Surface Studies and Department of Physics, University of Wisconsin-Milwaukee, Milwaukee, Wisconsin 53201 (United States)

The first observation of spin-dependent photoelectron diffraction using circularly polarized x rays is reported for monolayer ferromagnetic fcc Fe films on Cu(001). Circularly polarized x rays are used to produce spin-polarized photoelectrons from the Fe2[ital p] spin-orbit split doublet, and intensity asymmetries in the 2[ital p]3/2 level of [approx]3% are observed. The asymmetry is dependent on the relative orientation of the x-ray polarization vector and the Fe magnetic moment. This spin-dependent technique promises the direct, element-specific determination not only of local atomic structure, but magnetic structure as well.

DOE Contract Number:
W-7405-ENG-48
OSTI ID:
6836554
Journal Information:
Journal of Applied Physics; (United States), Journal Name: Journal of Applied Physics; (United States) Vol. 76:10; ISSN JAPIAU; ISSN 0021-8979
Country of Publication:
United States
Language:
English