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In situ X-ray absorption spectroscopy characterization of V{sub 2}O{sub 5} xerogel cathodes upon lithium intercalation

Journal Article · · Journal of the Electrochemical Society
DOI:https://doi.org/10.1149/1.1391946· OSTI ID:680036
; ;  [1]; ; ;  [2]
  1. Univ. of Minnesota, Minneapolis, MN (United States)
  2. Brookhaven National Lab., Upton, New York (United States)

Vanadium pentoxide materials prepared through sol-gel processes act as excellent intercalation hosts for lithium as well as for polyvalent cations. Previous ex situ X-ray absorption spectroscopy and X-ray diffraction characterizations have shown that the electrochemical performance of vanadium pentoxide xerogels depends inversely on the long-range order of the V{sub 2}O{sub 5}-layered structure. Recently, new ways to prevent the self-organization of the dry materials, which takes place upon water removal from the starting hydrogel, have been introduced. In the present paper the authors report on the in situ X-ray absorption spectroscopy characterization of a spray-coated V{sub 2}O{sub 5} (freeze-dried) xerogel cathode upon lithium intercalation.

Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY
Sponsoring Organization:
USDOE, Washington, DC (United States)
DOE Contract Number:
FG02-93ER14384; AC02-98CH10886
OSTI ID:
680036
Journal Information:
Journal of the Electrochemical Society, Journal Name: Journal of the Electrochemical Society Journal Issue: 7 Vol. 146; ISSN JESOAN; ISSN 0013-4651
Country of Publication:
United States
Language:
English

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