Lasing in active, sub-mean-free path-sized systems with dense, random, weak scatterers
- Department of Physics, Indian Institute of Science, Bangalore 560012 (India)
- Raman Research Institute, Bangalore 560080 (India)
We report enhanced emission and gain narrowing in Rhodamine 590 perchlorate dye in an aqueous suspension of polystyrene microspheres. A systematic experimental study of the threshold condition for and the gain narrowing of the stimulated emission over a wide range of dye concentrations and scatterer number densities showed several interesting features, even though the transport mean free path far exceeded the system size. The conventional diffusive-reactive approximation to radiative transfer in an inhomogeneously illuminated random amplifying medium, which is valid for a transport mean-free path much smaller than the system size, is clearly inapplicable here. We propose a new probabilistic approach for the present case of dense, random, weak scatterers involving the otherwise rare and ignorable sub-mean-free-path scatterings, now made effective by the high gain in the medium, which is consistent with experimentally observed features. {copyright} 1997 Optical Society of America
- OSTI ID:
- 678695
- Journal Information:
- Applied Optics, Journal Name: Applied Optics Journal Issue: 30 Vol. 36; ISSN APOPAI; ISSN 0003-6935
- Country of Publication:
- United States
- Language:
- English
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