Reactivity bands in atom--molecule collisions. IV. Coplanar and 3D studies of T+HT
Journal Article
·
· J. Chem. Phys.; (United States)
The system T+HT, which showed collinear reactivity bands for T+HT..-->..TH+T, is studied in 1D, 2D, and 3D for all possible orientations. The energy range is 0--2 eV (c.m.). Two and three dimensional Monte Carlo studies show no evidence of bands in the total reaction probability. Coplanar reactivity maps are analyzed to explain why the bands disappear. It is shown that the region leading to multiple collisions occupies a very narrow portion of the total configuration space available to reactants. This region is masked by the large reactivity for nonlinear orientations. Some systems which may show more persistent banding effects are proposed.
- Research Organization:
- Department of Chemistry, Carleton University, Ottawa, Canada K1S 5B6
- OSTI ID:
- 6738675
- Journal Information:
- J. Chem. Phys.; (United States), Journal Name: J. Chem. Phys.; (United States) Vol. 69:2; ISSN JCPSA
- Country of Publication:
- United States
- Language:
- English
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Related Subjects
640304* -- Atomic
Molecular & Chemical Physics-- Collision Phenomena
74 ATOMIC AND MOLECULAR PHYSICS
ATOM COLLISIONS
ATOM-MOLECULE COLLISIONS
BETA DECAY RADIOISOTOPES
BETA-MINUS DECAY RADIOISOTOPES
COLLISIONS
HYDROGEN ISOTOPES
HYDROGEN TRITIDE
ISOTOPES
KINETICS
LABELLED COMPOUNDS
LIGHT NUCLEI
MOLECULE COLLISIONS
MONTE CARLO METHOD
NUCLEI
ODD-EVEN NUCLEI
RADIOISOTOPES
REACTION KINETICS
TRITIUM
TRITIUM COMPOUNDS
YEARS LIVING RADIOISOTOPES
Molecular & Chemical Physics-- Collision Phenomena
74 ATOMIC AND MOLECULAR PHYSICS
ATOM COLLISIONS
ATOM-MOLECULE COLLISIONS
BETA DECAY RADIOISOTOPES
BETA-MINUS DECAY RADIOISOTOPES
COLLISIONS
HYDROGEN ISOTOPES
HYDROGEN TRITIDE
ISOTOPES
KINETICS
LABELLED COMPOUNDS
LIGHT NUCLEI
MOLECULE COLLISIONS
MONTE CARLO METHOD
NUCLEI
ODD-EVEN NUCLEI
RADIOISOTOPES
REACTION KINETICS
TRITIUM
TRITIUM COMPOUNDS
YEARS LIVING RADIOISOTOPES