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Natural radionuclides in groundwaters

Conference ·
OSTI ID:6700305
The U-234 and Th-230 radionuclides are highly retarded by factors of 10{sup 4} to 10{sup 5} in basalt groundwater (Hanford) and briny groundwaters from Texas and geothermal brine from the Salton Sea Geothermal Field (SSGF). In basalt groundwaters (low ionic strength), Ra is highly sorbed, while in brines (high ionic strength), Ra is soluble. This is probably because the sorption sites are saturated with Na{sup +} and Cl{sup {minus}} ions and RaCl{sub 2} is soluble in brines. Pb-210 is soluble in SSGF brine, probably as a chloride complex. The U-234/Th-230 ratios in basalt groundwaters and brines from Texas and SSGF are nearly unity, indicating that U is in the +4 state, suggesting a reducing environment for these aquifers. 19 refs., 3 figs.
Research Organization:
Pacific Northwest Lab., Richland, WA (USA)
Sponsoring Organization:
DOE/ER
DOE Contract Number:
AC06-76RL01830
OSTI ID:
6700305
Report Number(s):
PNL-SA-17438; CONF-900125--1; ON: DE90015286
Country of Publication:
United States
Language:
English

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