Growth of high phasematched temperature LiNbO/sub 3/ single crystals and application to efficient second harmonic generation of Nd:YAG. Final report
It was demonstrated that LiNbO/sub 3/ crystals with a phasematching temperature greater than 180/sup 0/C can be grown with small concentration gradients from a melt doped with MgO and excess Li/sub 2/O together with a planar growth interface; that the phasematch temperature can be readily adjusted simply by changing the excess Li/sub 2/O concentration proportional to the phasematch temperature desired; that the crystal quality and SHG characteristics can be maintained as long as the MgO concentration and growth parameters are held constant. We have also found that the self-annealing temperature is much lower, near 120/sup 0/C for the Stanford grown crystals, as compared to the previously reported value of 170 to 180/sup 0/C. Taking advantage of the lower self-annealing temperature, the crystals grown with phasematching temperature of approximately 120/sup 0/C showed exceptional optical homogeneity, and a 40% average power SHG conversion efficiency. The improved hot phasematching LiNbO/sub 3/ crystals along with the electro-optical or piezo-optical compensation for self heating effects should greatly enhance crystal device applications to high average power second harmonic generation of the Nd:YAG source.
- Research Organization:
- Stanford Univ., CA (USA). Center for Materials Research
- DOE Contract Number:
- W-7405-ENG-48
- OSTI ID:
- 6690806
- Report Number(s):
- UCRL-15310
- Country of Publication:
- United States
- Language:
- English
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OPTICAL PROPERTIES
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NIOBATES
CRYSTAL GROWTH
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MONOCRYSTALS
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CHALCOGENIDES
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420300* - Engineering- Lasers- (-1989)