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The thermodynamic properties of thianthrene and phenoxathiin

Technical Report ·
DOI:https://doi.org/10.2172/6673493· OSTI ID:6673493

Measurements leading to the calculation of the ideal-gas thermodynamic properties are reported for thianthrene (Chemical Abstracts registry number [92-85-3]) and phenoxathiin (registry number [262-20-41]). Experimental methods included combustion calorimetry, adiabatic heat-capacity calorimetry, vibrating-tube densitometry, comparative ebulliometry, inclined-piston gauge manometry, and differential-scanning calorimetry (d.s.c.). Critical properties were estimated for both materials based on the measurement results. Entropies, enthalpies, and Gibbs energies of formation were derived for the ideal gas for both compounds for selected temperatures between 298.15 K and 700 K. The property-measurement results reported here for thianthrene and phenoxathiin provide the first experimental gas-phase Gibbs energies of formation for tricyclic diheteroatom-containing molecules.

Research Organization:
National Inst. for Petroleum and Energy Research, Bartlesville, OK (United States)
Sponsoring Organization:
DOE; USDOE, Washington, DC (United States)
DOE Contract Number:
FC22-83FE60149
OSTI ID:
6673493
Report Number(s):
NIPER-659; ON: DE93000124
Country of Publication:
United States
Language:
English