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Helium permeability of BISO high-temperature gas-cooled reactor (HTGR) fuel particles

Technical Report ·
OSTI ID:6612795
The permeabilities of helium through the pyrocarbon coatings of BISO HTGR fuel particle Batches OR2263HT, OR2269HT, J596, J598, J605, and J606 prepared by the Metals and Ceramics Division, Oak Ridge National Laboratory have been measured over the temperature range of 450 to 1200/sup 0/C. These measurements were analyzed in terms of a simple diffusion model whereby the porosity of the pyrocarbon coating, the frequency factor term for diffusion (D/sub 0/), and the activation energy for diffusion were determined. The batch-to-batch variations in permeability ranged over a factor of 57 from the least permeable (J596) to the most permeable (J598). The major contribution to this variability was D/sub 0/ (1 x 10/sup -7/ to 5 x 10/sup -6/ m/sup 2/s/sup -1/) with porosity (1 to 5%) being second most important. The activation energy for diffusion (103 to 123 Kj mol/sup -1/) displayed the least effect (approximately a factor of 2) on the batch-to-batch variability in the helium permeability.
Research Organization:
Oak Ridge Y-12 Plant, TN (USA)
DOE Contract Number:
W-7405-ENG-26
OSTI ID:
6612795
Report Number(s):
Y/DA-8035
Country of Publication:
United States
Language:
English