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Title: Measurement of fission neutron multiplicities for thorium-232 and uranium-235 with incident neutron energies to 49 MeV

Journal Article · · Nucl. Sci. Eng.; (United States)
OSTI ID:6581073

Fission neutron multiplicities have been measured for neutrons incident on /sup 232/Th with energies ranging from 1.1 to 49 MeV and for neutrons incident on /sup 235/U with energies from 17 to 49 MeV. The Lawrence Livermore National Laboratory 100-MeV electron Linac was used to produce a white source of neutrons. Incident neutron energies were measured using time-of-flight techniques. Fission neutrons were detected in a liquid scintillator using pulse-shape discrimination. All /sup 232/Th neutron multiplicities were measured relative to /sup 235/U at each incident neutron energy. Above 15 MeV the multiplicities were determined for /sup 232/Th and /sup 235/U by using lower energy data from the /sup 235/U sample to measure the neutron detector efficiency. Corrections for angular anisotropy and spectral temperatures of the fission neutrons were minimized through the use of a spherical shell of /sup 235/U surrounding the fission chamber. The present results for /sup 232/Th extend available multiplicity data into the previously unreported regions: 1.1 to 1.3 MeV and 17 to 49 MeV. The /sup 235/U results also extend significantly beyond previously reported data. For the /sup 232/Th case, previously observed deviations from linearity below 2 MeV and near the (n, n'f) threshold have been confirmed. In addition, this experiment suggests a continued rise in neutron multiplicity with decreasing incident neutron energy down to 1.1 MeV. A value for /sup -/v /SUB p/ of /sup 231/Th(n,f) is inferred from the /sup 232/Th results above the (n, n'f) threshold. The /sup 232/Th measurements reported here for neutron energies above 15 MeV show an average value of dE /SUB n/ /d/sup -/v /SUB p/, which agrees with a value calculated from the binding energies of the pre-scission evaporated neutrons and the assumed mean kinetic energies. The /sup 235/U data do not exhibit such a close agreement.

Research Organization:
University of California, Lawrence Livermore National Laboratory Livermore, California
OSTI ID:
6581073
Journal Information:
Nucl. Sci. Eng.; (United States), Vol. 86:2
Country of Publication:
United States
Language:
English

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