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Optical Raman heterodyne detection of /sup 27/Al superhyperfine spectra in ruby

Journal Article · · Opt. Lett.; (United States)
DOI:https://doi.org/10.1364/OL.13.001075· OSTI ID:6574899
We report extension of the Raman heterodyne technique for detection of nuclear magnetic resonance (NMR) to superhyperfine spectra. NMR of the four nearest neighbor sets of /sup 27/Al (I = 5/2) surrounding Cr/sup 3+/ in ruby has been observed with high sensitivity using optical excitation of the R/sub 1/ line at 693.4 nm. Either excited-state or ground-state resonances could be selectively displayed by setting the sample temperature to 2 or 7.5 K, respectively. All 40 expected NMR resonances were observed, with good agreement obtained between calculated and experimental values.
Research Organization:
Division of Physics, National Research Council of Canada, Ottawa, Ontario, Canada K1A 0R6
OSTI ID:
6574899
Journal Information:
Opt. Lett.; (United States), Journal Name: Opt. Lett.; (United States) Vol. 13:12; ISSN OPLED
Country of Publication:
United States
Language:
English