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Hanford derived plutonium in Columbia River sediments

Technical Report ·
OSTI ID:6539694

Mass spectrometry analyses of Pu isolated from Columbia River sediments exhibit mean Pu 240/242 ratios consistent with those observed for integrated global fallout. Pu 240/239 ratios show marked deviations from accepted fallout values arguing for a second source of Pu-239. This additional Pu-239 arises from the decay Np-239 produced in reactor effluent water from the old Pu production reactors located on the Hanford Reservation. An estimated 20 to 25 percent of the total Pu inventory in sediments behind McNary Reservoir, the first down-river site of fine sediment accumulation below the Hanford Reservation, are ascribed to reactor operations.

Research Organization:
Oregon State Univ., Newport (USA). Marine Science Center; Du Pont de Nemours (E.I.) and Co., Aiken, SC (USA). Savannah River Lab.
DOE Contract Number:
AT06-76EV70030
OSTI ID:
6539694
Report Number(s):
DOE/EV/70030-6
Country of Publication:
United States
Language:
English

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