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Solution softening in spinel

Journal Article · · Scripta Materialia
 [1];  [2];  [3]
  1. Los Alamos National Lab., NM (United States). Center for Materials Science
  2. Ford Motor Co., Dearborn, MI (United States). Scientific Research Lab.
  3. Case Western Reserve Univ., Cleveland, OH (United States). Dept. of Materials Science and Engineering

Conclusions from this study are: 1. The critical resolved shear stress of MgO.nAl{sub 2}O{sub 3} spinel at a given temperature decreases dramatically, by almost two orders of magnitude, with increasing deviation form stoichiometry, i.e., as n increases from 1 to 3.5. 2. The CRSS is proportional to exp({minus}T/T{sub 0}) and to [V{sub c}]{sup {minus}2}, where T{sub 0} is a characteristic temperature and [V{sub c}] is the concentration of charge-compensating cation vacancies. 3. Slip on {l_brace}111{r_brace} planes is thought to occur between the Kagome cation Layers and the adjacent anion layers. Slip on {l_brace}101{r_brace} planes is slightly easier (and has a higher T{sub 0}) because the planes are more widely separated. 4. Slip in spinel does not require synchro-shear, unlike slip in the C15 AB{sub 2} Laves phase, which has identical metal atom positions to the cation positions in spinel. 5. The temperature dependence of the CRSS is analyzed in terms of a model based on partial dislocations overcoming a steep and high Peierls potential. Parameters for the model can be chosen to explain the observed values of T{sub 0} and the CRSS extrapolated to T = 0 K for both spinel and sapphire. Other models are possible. 6. The dependence of CRSS on [V{sub c}]{sup {minus}2} can be explained in terms of kink nucleation at cation vacancies.

Sponsoring Organization:
USDOE, Washington, DC (United States)
OSTI ID:
651149
Report Number(s):
CONF-980202--
Journal Information:
Scripta Materialia, Journal Name: Scripta Materialia Journal Issue: 4-5 Vol. 39; ISSN 1359-6462; ISSN SCMAF7
Country of Publication:
United States
Language:
English

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