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Energy-loss calculations for medium-energy rare gas+H/sub 2/ collision

Journal Article · · Phys. Rev. A; (United States)
Cross sections differential in energy loss and scattering angle and most-probable reciprocal-mass functions are calculated for several rare gases on H/sub 2/ collisions i the low-keV collision-energy range. Specifically, the collision systems He+H/sub 2/, Ne+H/sub 2/, and Ne/sup +/+H/sub 2/ have been considered. The classical-trajectory calculations are based on a triatomic-molecular potential-functional form suggested by ab initio calculations of the He-H/sub 2/ energy He-H/sub 2/ energy surface, which serves as a prototype for all rare-gas-H/sub 2/ systems. The parameters in that functional form have been fitted from the experimental differential energy-loss measurements for Ne on H/sub 2/ collisions to yield the Ne-H/sub 2/ energy surface, and from the Ne/sup +/ on H/sub 2/ differential energy-loss measurements to yield the Ne-H/sub 2//sup +/ energy surface. With the energy surfaces thus parametrized, the calculated differential energy-loss cross sections agree well with the experimental data. They explain the anomalously large range of scattering angle in which the collision is elastic, with no vibrational-rotational excitation.
Research Organization:
Department of Physics, University of Connecticut, Storrs, Connecticut 06268
OSTI ID:
6510876
Journal Information:
Phys. Rev. A; (United States), Journal Name: Phys. Rev. A; (United States) Vol. 26:4; ISSN PLRAA
Country of Publication:
United States
Language:
English