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Experimental evaluation of catalytic combustion with heat removal at near stoichiometric conditions

Conference ·
OSTI ID:6509998
Two concentric tube configurations were tested to evaluate catalytic combustion with heat removal at near stoichiometric conditions. Tests were conducted at an inlet pressure of 1.5x10/sup 5/Pa, inlet fuel-air mixture temperatures from 780 to 960 K, combustion air flow rates from 0.78 to 1.5 g/s, equivalence ratios up to 0.90, and a range of cooling air flow rates. Propane and propylene fuels were used. Both configurations used air flowing through the center tube for cooling and combustion in the annulus on the catalytic surface. One configuration had the catalyst applied to the outside surface of the inner tube. Conversion of the fuel was very low for this configuration. At an inlet fuel-air mixture temperature of 960/sup 0/K, a combustion air flow rate of 1.5 g/s, an inlet velocity of 11 m/s, and a propylene fuel flow rate of 6.0x10/sup -2/ g/s, 34% of the heat available from the fuel was transferred to the cooling air in the center tube using a platinum catalyst. The other configuration had the catalyst applied to the inside surface of the outer tube. Conversion of the fuel was considerably better in this configuration. At an inlet mixture temperature of 925/sup 0/K, a combustion air flow rate of 1.0 g/s, an inlet velocity of 22 m/s, and propylene fuel flow rate of 6.0x10/sup -2/ g/s, 58% of the heat available from the fuel was transferred to the cooling air in the inner tube using a platinum/rhodium catalyst. At equivalence ratios as high as 0.87, NO/sub x/ emissions less than 0.2 g NO/sub 2//kg fuel were obtained. Combustion efficiencies greater than 99.5% were measured for certain operating conditions with this configuration.
Research Organization:
National Aeronautics and Space Administration, Cleveland, OH (USA). Lewis Research Center
DOE Contract Number:
AI01-77CS51040
OSTI ID:
6509998
Report Number(s):
DOE/NASA/51040-23; CONF-800553-3; NASA-TM-81748
Country of Publication:
United States
Language:
English