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Fast neutron inelastic scattering cross sections in /sup 232/Th

Thesis/Dissertation ·
OSTI ID:6495146

Fast neutron inelastic scattering cross sections for levels between 700-1550-keV excitation energy in the actinide nucleus, /sup 232/Th, have been measured using the (n,n') time-of-flight technique. Two series of measurements were undertaken using neutrons with a typical energy spread of 8-10 keV, generated by the /sup 7/Li(p,n)/sup 7/Be reaction. These measurements for 125/sup 0/ -differential scattering cross sections were performed over the incident neutron energy regions of 1) 0.950-1.550 MeV, in 50-keV intervals with the time-of-flight spectrometer optimized to detect 0.200-0.400-MeV scattered neutrons and 2) 1.200-2.000 MeV, in 100-keV intervals with the time-of-flight spectrometer optimized to detect 0.400-0.800-MeV scattered neutrons. Techniques for unfolding the complicated spectra obtained from these (n,n') studies were developed, employing user interactive computer codes. Excitation function and angular distribution results were compared with 1) theoretical calculations that included both compound-nucleus and direct-interaction mechanisms, 2) the Evaluated Nuclear Data File (ENDF-B/V) and 3) previous (n,n') and (n,n'..gamma..) cross section measurements. Where applicable, estimates of electric monopole (EO) transition strengths were determined from these comparisons.

Research Organization:
Lowell Univ., MA (USA)
OSTI ID:
6495146
Country of Publication:
United States
Language:
English