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Characterization of the thermally contracting tungstates Ta/sub 22/W/sub 4/O/sub 67/, Ta/sub 2/WO/sub 8/, and Ta/sub 16/W/sub 18/O/sub 94/

Journal Article · · J. Am. Ceram. Soc.; (United States)

An investigation of the properties of high-purity (> 99 wt %) tantalum tungstates (Ta/sub 22/W/sub 4/O/sub 67/, Ta/sub 2/WO/sub 8/, and Ta/sub 16/W/sub 18/O/sub 94/) included determination of density (bulk and theoretical), refined lattice constants, maximum use temperatures, microhardness, heat capacity, thermal expansion (contraction) and diffusivity, calculated thermal conductivity, and electrical resistivity. Usable to approx. = 1700 K in air or inert atmospheres, these tantalum tungstates have theoretical densities of 7.3 to 8.5 g/cm/sup 3/, are relatively soft (120 to 655 kg/mm/sup 2/ hardnesses), and are electrical insulators (6 x 10/sup 3/ to 2 x 10/sup 8/ ..cap omega...cm resistivities). The distinguishing properties of the materials are their thermal expansion (average CTE values from +0.6 x 10/sup -6//K to -5.1 x 10/sup -6//K at 293 to 1273 K), thermal expansion hysteresis with minimal observable microcracking, and thermal diffusivity (values from 1.6 x 10/sup -3/ to 3.2 x 10/sup -3/ cm/sup 2//s at 298 K) gradually increasing with temperature.

Research Organization:
Oak Ridge Y-12 Plant, TN
OSTI ID:
6464027
Journal Information:
J. Am. Ceram. Soc.; (United States), Journal Name: J. Am. Ceram. Soc.; (United States) Vol. 61:3-4; ISSN JACTA
Country of Publication:
United States
Language:
English