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NO/NO2/O3 photostationary state in Claremont, California

Journal Article · · J. Air Pollut. Control Assoc.; (United States)

Seventeen days of detailed measurements of NO, NO2, O3, HNO3 and the frequency of NO2 photolysis - j(NO2) - were carried out in Claremont, CA, in September 1980. Under conditions when the rate of change of NO concentration is small, there must be a balance between formation and loss processes. In the classical photostationary state this balance is between NO2 photolysis: NO2 + hv yields NO + O and reaction with ozone: NO + O3 yields NO2 + O2. The results show that the latter reaction with ozone is inadequate to balance the formation step a significant contribution is required from another NO oxidation process, possibly peroxy radical oxidation. If so, the inferred concentration of peroxy radicals shows a diurnal variation, peaking around solar noon.

Research Organization:
Michigan Univ., Ann Arbor
OSTI ID:
6445304
Journal Information:
J. Air Pollut. Control Assoc.; (United States), Journal Name: J. Air Pollut. Control Assoc.; (United States) Vol. 33; ISSN JPCAA
Country of Publication:
United States
Language:
English